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Homogeneity of Continuum Model of an Unsteady State Fixed Bed Reactor for Lean CH4 Oxidation
Subagjo1, Yogi Wibisono Budhi1*, M. Effendy1 & Yazid Bindar2
1Research Group of Chemical Engineering Process Design and Development Faculty of Industrial Technology, Institut Teknologi Bandung, Jalan Ganesha 10, Bandung 40132, Indonesia
2Research Group of Chemical Engineering Energy and Processing System, Faculty of Industrial Technology, Institut Teknologi Bandung, Jalan Ganesha 10, Bandung 40132, Indonesia
*Email: Y.Wibisono@che.itb.ac.id
Abstract. In this study, the homogeneity of the continuum model of a fixed bed reactor operated in steady state and unsteady state systems for lean CH4 oxidation is investigated. The steady-state fixed bed reactor system was operated under once-through direction, while the unsteady-state fixed bed reactor system was operated under flow reversal. The governing equations consisting of mass and energy balances were solved using the FlexPDE software package, version 6. The model selection is indispensable for an effective calculation since the simulation of a reverse flow reactor is time-consuming. The homogeneous and heterogeneous models for steady state operation gave similar conversions and temperature profiles, with a deviation of 0.12 to 0.14%. For reverse flow operation, the deviations of the continuum models of thepseudo-homogeneous and heterogeneous models were in the range of 25-65%. It is suggested that pseudo-homogeneous models can be applied to steady state systems, whereas heterogeneous models have to be applied to unsteady state systems.
Keywords: continuum model; mathematical modeling; methane; oxidation; reverse flow reactor; simulation.
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